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Journal Articles

Hierarchical aggregation in a complex fluid; The Role of isomeric interconversion

Massey, D.*; Williams, C. D.*; Mu, J.*; Masters, A. J.*; Motokawa, Ryuhei; Aoyagi, Noboru; Ueda, Yuki; Antonio, M. R.*

Journal of Physical Chemistry B, 127(9), p.2052 - 2065, 2023/03

 Times Cited Count:0 Percentile:0(Chemistry, Physical)

Journal Articles

Nature of isomerism in exotic sulfur isotopes

Utsuno, Yutaka; Shimizu, Noritaka*; Otsuka, Takaharu*; Yoshida, Toru*; Tsunoda, Yusuke*

Physical Review Letters, 114(3), p.032501_1 - 032501_5, 2015/01

AA2014-0621.pdf:0.23MB

 Times Cited Count:37 Percentile:85.32(Physics, Multidisciplinary)

In usual even-even nuclei, $$0^+_1$$, $$2^+_1$$, $$4^+_1cdots$$ states are known to be connected via strong $$E2$$ transitions. The recently observed $$4^+_1$$ state in the neutron-rich nucleus $$^{44}$$S has a strongly hindered $$E2$$ transition to the $$4^+_1$$ state. We report the origin of this strong hindrance in this paper. While shell-model calculations reproduce the hindrance, their many-body wave functions are too complicated for one to understand the nature. In this study, we introduce a novel method to obtain wave functions in the intrinsic frame by performing the variation after angular-momentum projection. The $$0^+_1$$, $$2^+_1$$ states are dominated by the usual $$K=0$$ state, whereas for the $$4+$$ level the $$K=4$$ state is lower than $$K=0$$ state, which causes the $$E2$$ hindrance. We also account for similar $$E2$$ hindrance in $$^{43}$$S in this framework. The $$4^+$$ level is the lightest-mass high-$$K$$ isomer ever found.

Journal Articles

Revaluation of the correlation of isomer shift with Np-O bond length in various neptunyl(V and VI) compounds

Saeki, Masakatsu; Nakada, Masami; Kawasaki, Takeshi*; Nishimura, Tatsuru*; Kitazawa, Takafumi*; Takeda, Masuo*

Journal of Radioanalytical and Nuclear Chemistry, 270(2), p.379 - 384, 2006/11

 Times Cited Count:3 Percentile:24.08(Chemistry, Analytical)

no abstracts in English

Journal Articles

Identification of the $$K^pi=11/2^+$$ isomer in neutron-rich $$^{187}$$W

Shizuma, Toshiyuki; Hayakawa, Takehito; Mitarai, Shiro*; Morikawa, Tsuneyasu*; Ishii, Tetsuro

Physical Review C, 71(6), p.067301_1 - 067301_4, 2005/06

 Times Cited Count:6 Percentile:45.52(Physics, Nuclear)

Excited states in neutron-rich $$^{187}$$W have been populated via deep inelastic collisions of a 630-MeV $$^{82}$$Se beam on a $$^{186}$$W target. Projectile-like fragments were measured by an annular Si detector for reaction channel selection. Delayed $$gamma$$ rays from target residues were detected by means of the so-called recoil shadow technique. A new isomer at 411 keV, based on the $$11/2^+$$[615] Nilsson configuration, has been identified with the half-life of 1.56(28) $$mu$$s. The decay rates of the isomers are discussed in terms of the $$K$$ quantum number by comparison with the systematics from the neighboring nuclei.

Journal Articles

Correlation between $$^{237}$$Np M$"o$essbauer parameter and crystal structure of neptunyl compounds

Saeki, Masakatsu

Nihon Kessho Gakkai-Shi, 46(6), p.415 - 420, 2004/12

no abstracts in English

Journal Articles

A New isomer in $$^{136}$$Ba populated by deep inelastic collisions

Shizuma, Toshiyuki; Gan, Z. G.*; Ogawa, Kengo*; Nakada, Hitoshi*; Oshima, Masumi; Toh, Yosuke; Hayakawa, Takehito; Hatsukawa, Yuichi; Sugawara, Masahiko*; Utsuno, Yutaka; et al.

European Physical Journal A, 20(2), p.207 - 210, 2004/04

 Times Cited Count:13 Percentile:71.74(Physics, Nuclear)

Excited states in $$^{136}$$Ba, populated in deep-inelastic collisions by the interaction of 450-MeV $$^{82}$$Se ions with a $$^{139}$$La target, have been studied by means of in-beam $$gamma$$-ray spectroscopy. A new isomer with $$I^pi=(10^+)$$ has been identified at an excitation energy of $$E_x=3.357$$ MeV. The half-life was determined as $$T_{1/2}=94pm10$$ ns. The extracted $$B(E2)$$ value is much smaller than those in $$^{132}$$Te and $$^{134}$$Xe. This hindrance is investigated by a shell model calculation.

Journal Articles

Relationship between M$"o$ssbauer Isomer shifts and Structures of Neptunium compounds

Saeki, Masakatsu; Nakada, Masami; Kitazawa, Takafumi*

KURRI-KR-106, p.38 - 42, 2004/03

no abstracts in English

Journal Articles

High-spin structure in $$^{185}$$Os

Shizuma, Toshiyuki; Mitarai, Shiro*; Sletten, G.*; Bark, R. A.*; Gjorup, N. L.*; Jensen, H. J.*; Piiparinen, M.*; Wrzesinski, J.*; Shimizu, Yoshifumi*

Physical Review C, 69(2), p.024305_1 - 024305_18, 2004/02

 Times Cited Count:15 Percentile:65.29(Physics, Nuclear)

High-spin states in $$^{185}$$Os have been studied using the $$^{176}$$Yb($$^{13}$$C,4n) reaction at a beam energy of 65MeV. Previously known 1-quasiparticle bands have been extended to higher spins. New high-$$K$$ bands based on 3- and 5-quasiparticle excitation have been identified. Nilsson configurations are assigned based on the g-factors deduced from M1/E2 branching ratios within the bands. In addition, a new isomer at 5008keV has been found with a half-life of 18(2) ns. The hindrance in decays of the high-$$K$$ intrinsic states are discussed in terms of the $$gamma$$ tunneling model where the low-$$K$$ and high-$$K$$ states interact through the triaxial shape fluctuation.

Journal Articles

${it Trans}$-1,2-dichloroethylene decomposition in low-humidity air under electron beam irradiation

Sun, Y.*; Hakoda, Teruyuki; Chmielewski, A. G.*; Hashimoto, Shoji*

Radiation Physics and Chemistry, 68(5), p.843 - 850, 2003/12

 Times Cited Count:8 Percentile:49.8(Chemistry, Physical)

no abstracts in English

Journal Articles

Inelastic excitation of $$^{187}$$Re

Shizuma, Toshiyuki; Toh, Yosuke; Oshima, Masumi; Sugawara, Masahiko*; Matsuda, Makoto; Hayakawa, Takehito; Koizumi, Mitsuo; Osa, Akihiko; Zhang, Y. H.*; Liu, Z.*

European Physical Journal A, 17(2), p.159 - 165, 2003/06

 Times Cited Count:10 Percentile:55.54(Physics, Nuclear)

High-spin states in $$^{187}$$Re populated by inelastic scattering of a 500-MeV $$^{82}$$Se beam have been studied by means of in-beam $$gamma$$-ray spectroscopy. Levels built on the $$5/2^+$$[402] and $$9/2^-$$[514] one-quasiparticle states were measured up to $$I^pi=(21/2^+)$$ and $$(21/2^-)$$, respectively. In additions, several new levels including an isomer at 1682 keV with a half-life of 114(23) ns have been found. Quasiparticle configurations of the levels and the transition rates are discussed.

Journal Articles

Neutron capture cross section to $$^{186}$$Re isomeric state

Hayakawa, Takehito; Shizuma, Toshiyuki; Yamauchi, Toshihiko; Minehara, Eisuke; Arisawa, Takashi

Nuclear Physics A, 718, p.665c - 667c, 2003/05

no abstracts in English

Journal Articles

$$^{151}$$Eu M$"o$ssbauer spectroscopic study on the Eu$$_{y}$$M$$_{1-y}$$O$$_{2-y}$$(0$$leq$$y$$leq$$1.0)(M=Th, U)

Masaki, Nobuyuki; Otobe, Haruyoshi; Nakamura, Akio; Harada, Daijitsu*; Ito, Kentaro*; Sasaki, Yoshinobu*; Hinatsu, Yukio*

Journal of Nuclear Science and Technology, 39(Suppl.3), p.217 - 220, 2002/11

no abstracts in English

Journal Articles

Tunneling in high-$$K$$ isomeric decays

Shizuma, Toshiyuki; Shimizu, Yoshifumi*; Hayakawa, Takehito

Journal of Nuclear Science and Technology, 39(11), p.1137 - 1141, 2002/11

 Times Cited Count:4 Percentile:29.2(Nuclear Science & Technology)

We have systematically investigated the highly $$K$$-forbidden transitions observed in the Hf, W and Os region, using the $$gamma$$-tunneling model in which low-$$K$$ and high-$$K$$ states interact through a process of the quantum tunneling. In the present study, we have analyzed $$K$$-forbidden transitions recently observed. The measured hindrance factors are compared with the values calculated using the $$gamma$$-tunneling model. We have also investigated isotope dependences of $$gamma$$ tunneling probabilities particularly for neutron-rich nuclei.

Journal Articles

High-$$K$$ negative parity states in $$^{184}$$Os

Shizuma, Toshiyuki; Stevenson, P. D.*; Walker, P. M.*; Toh, Yosuke; Hayakawa, Takehito; Oshima, Masumi; Furuno, Kohei*; Komatsubara, Tetsuro*

Physical Review C, 65(6), p.064310_1 - 064310_12, 2002/06

 Times Cited Count:15 Percentile:62.86(Physics, Nuclear)

High-spin states in $$^{184}$$Os have been studied using the $$^{170}$$Er($$^{18}$$O,4n) reaction at a beam energy of 85 MeV. Several new negative parity levels including a 48-ns $$K^pi=(18^-)$$ isomer have been identified. Nilsson configurations for the levels are assigned by comparison with multi-quasiparticle calculations. Potential-energy-surface calculations show an increasing influence of triaxiality in nuclear shapes at higher spins. The decay rate of the $$K^pi=(18^-)$$ isomer is discussed in relation to the role of the $$K$$ quantum number.

Journal Articles

Multi-quasiparticle states and ${it K}$-forbidden transitions in $$^{183}$$Os

Shizuma, Toshiyuki; Matsuura, Katsuyuki*; Toh, Yosuke; Hayakawa, Takehito; Oshima, Masumi; Hatsukawa, Yuichi; Matsuda, Makoto; Furuno, Kohei*; Sasaki, Yasuyuki*; Komatsubara, Tetsuro*; et al.

Nuclear Physics A, 696(3-4), p.337 - 370, 2001/12

 Times Cited Count:20 Percentile:73.8(Physics, Nuclear)

High-spin states in $$^{183}$$Os have been studied using the 170Er(18O,5n) reaction at a beam energy of 85 MeV. Nine rotational bands based on 1-, 3-, 5- and 7-quasiparticle excitations have been observed. Nilsson configurations are assigned for the newly observed bands using g-factors deduced from M1/E2 branching ratios within the bands. In addition, two isomers with K=(43/2+) and (43/2-) have been identified. The K=(43/2+) isomer decays directly to the K=9/2+ ground state band with a large difference in the $$K$$ quantum number, $$mitDelta K=$$17. The decay rates are disccused in terms of a tunneling model where high-$$K$$ (isomeric) and low-$$K$$ states interact via fluctuations towards triaxial nuclear shapes.

Journal Articles

The Spartial effect of hydrophobic groups in pendant amino acid monomers on the thermal volume phase transition of hydrogels

Hendri, J.*; Hiroki, Akihiro*; Maekawa, Yasunari; Yoshida, Masaru; Katakai, Ryoichi*

Radiation Physics and Chemistry, 61(2), p.155 - 161, 2001/05

 Times Cited Count:2 Percentile:19.6(Chemistry, Physical)

no abstracts in English

Journal Articles

Decomposition test of PCB by CO$$_{2}$$ laser irradiation

Yamauchi, Toshihiko; Kamei, Yasutaka*; Ito, Shinichi*; Furukawa, Yukio*; Minehara, Eisuke

Kankyo Kagakkai-Shi, 14(1), p.73 - 76, 2001/01

no abstracts in English

Journal Articles

Definitive evidence for the existence of a long-lived vinylidene radical cation, H$$_{2}$$C=C$$^{+}$$

Hayakawa, Shigeo*; *; Arakawa, Kazuo; Morishita, Norio

Journal of Chemical Physics, 110(6-8), p.2745 - 2748, 1999/02

 Times Cited Count:21 Percentile:55.26(Chemistry, Physical)

no abstracts in English

Journal Articles

A Correlation between isomer shifts of $$^{237}$$Np Moessbauer spectra and coordination numbers of Np atoms in neptunyl(V) compounds

Saeki, Masakatsu; Nakada, Masami; Nakamoto, Tadahiro*; Yamashita, Toshiyuki; ; Krot, N. N.*

Journal of Radioanalytical and Nuclear Chemistry, 239(2), p.221 - 225, 1999/00

 Times Cited Count:7 Percentile:49.64(Chemistry, Analytical)

no abstracts in English

Journal Articles

Present status of advanced photon science research program related to X-, and $$gamma$$-ray emission source development

Arisawa, Takashi; Matoba, Toru; Yamakawa, Koichi; Maruyama, Yoichiro; Sasuga, Tsuneo; Wakaida, Ikuo; Nakajima, Kazuhisa*; Sasaki, Akira; Minehara, Eisuke; Oshima, Masumi

Proc. of the 1st International Induced Gamma Emision Workshop, p.29 - 41, 1999/00

no abstracts in English

31 (Records 1-20 displayed on this page)